| 1 | Tue 10 Aug 2021 | 274-0 v Peterborough UnitedPeterborough United 0-4 Plymouth Argyle | Carabao Cup First Round |
| 2 | Tue 17 Aug 2021 | 271-1 v Cambridge UnitedPlymouth Argyle 1-1 Cambridge United | Sky Bet League One |
| 3 | Sat 21 Aug 2021 | 273-0 v Shrewsbury TownShrewsbury Town 0-3 Plymouth Argyle | Sky Bet League One |
| 4 | Tue 24 Aug 2021 | 271-4 v Swansea CitySwansea City 4-1 Plymouth Argyle | Carabao Cup Second Round |
| 5 | Sat 28 Aug 2021 | 271-1 v Fleetwood TownPlymouth Argyle 1-1 Fleetwood Town | Sky Bet League One |
| 6 | Tue 31 Aug 2021 | 270-2 v Newport CountyNewport County 2-0 Plymouth Argyle | Papa John’s Trophy |
| 7 | Sat 11 Sep 2021 | 273-0 v Sheffield WednesdayPlymouth Argyle 3-0 Sheffield Wednesday | Sky Bet League One |
| 8 | Sat 18 Sep 2021 | 271-0 v AFC WimbledonAFC Wimbledon 0-1 Plymouth Argyle | Sky Bet League One |
| 9 | Tue 21 Sep 2021 | 272-2 v PortsmouthPortsmouth 2-2 Plymouth Argyle | Sky Bet League One |
| 10 | Tue 28 Sep 2021 | 271-1 v Crewe AlexandraPlymouth Argyle 1-1 Crewe Alexandra | Sky Bet League One |
| 11 | Tue 12 Oct 2021 | 271-3 v Swindon TownPlymouth Argyle 1-3 Swindon Town | Papa John’s Trophy |
| 12 | Sun 5 Dec 2021 | 27 2-1 v RochdaleRochdale 1-2 Plymouth Argyle | Emirates FA Cup Second Round |
| 13 | Sat 8 Jan 2022 | 271-0 v Birmingham CityBirmingham City 0-1 Plymouth Argyle | Emirates FA Cup Third Round |
| 14 | Sat 15 Jan 2022 | 272-4 v Sheffield WednesdaySheffield Wednesday 4-2 Plymouth Argyle | Sky Bet League One |
| 15 | Sat 22 Jan 2022 | 271-2 v Lincoln CityPlymouth Argyle 1-2 Lincoln City | Sky Bet League One |
| 16 | Sat 5 Feb 2022 | 271-2 v ChelseaChelsea 2-1 Plymouth Argyle | Emirates FA Cup Fourth Round |
| 17 | Tue 8 Feb 2022 | 274-1 v Crewe AlexandraCrewe Alexandra 1-4 Plymouth Argyle | Sky Bet League One |
| 18 | Tue 15 Mar 2022 | 271-0 v PortsmouthPlymouth Argyle 1-0 Portsmouth | Sky Bet League One |
| 19 | Sat 2 Apr 2022 | 271-0 v Oxford UnitedPlymouth Argyle 1-0 Oxford United | Sky Bet League One |
| 20 | Sat 9 Apr 2022 | 270-0 v Burton AlbionBurton Albion 0-0 Plymouth Argyle | Sky Bet League One |
| 21 | Sat 30 Apr 2022 | 270-5 v Milton Keynes DonsPlymouth Argyle 0-5 Milton Keynes Dons | Sky Bet League One |
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