| 1 | Mon 16 Aug 2021 | 240-0 v GranadaVillarreal 0-0 Granada |
| 2 | Sat 21 Aug 2021 | 240-0 v EspanyolEspanyol 0-0 Villarreal |
| 3 | Sun 29 Aug 2021 | 242-2 v Atlético MadridAtlético Madrid 2-2 Villarreal |
| 4 | Wed 22 Sep 2021 | 24 4-1 v ElcheVillarreal 4-1 Elche |
| 5 | Sun 17 Oct 2021 | 241-2 v OsasunaVillarreal 1-2 Osasuna |
| 6 | Tue 26 Oct 2021 | 243-3 v CádizVillarreal 3-3 Cádiz |
| 7 | Sat 20 Nov 2021 | 241-1 v Celta VigoCelta Vigo 1-1 Villarreal |
| 8 | Sat 27 Nov 2021 | 241-3 v BarcelonaVillarreal 1-3 Barcelona |
| 9 | Sat 4 Dec 2021 | 240-1 v SevillaSevilla 1-0 Villarreal |
| 10 | Sun 12 Dec 2021 | 242-0 v Rayo VallecanoVillarreal 2-0 Rayo Vallecano |
| 11 | Sat 18 Dec 2021 | 243-1 v Real SociedadReal Sociedad 1-3 Villarreal |
| 12 | Tue 21 Dec 2021 | 245-2 v AlavésVillarreal 5-2 Alavés |
| 13 | Sun 9 Jan 2022 | 242-2 v Atlético MadridVillarreal 2-2 Atlético Madrid |
| 14 | Sun 16 Jan 2022 | 240-1 v ElcheElche 1-0 Villarreal |
| 15 | Sat 22 Jan 2022 | 243-0 v MallorcaVillarreal 3-0 Mallorca |
| 16 | Sun 6 Feb 2022 | 242-0 v Real BetisReal Betis 0-2 Villarreal |
| 17 | Sat 12 Feb 2022 | 240-0 v Real MadridVillarreal 0-0 Real Madrid |
| 18 | Sat 19 Feb 2022 | 244-1 v GranadaGranada 1-4 Villarreal |
| 19 | Sat 12 Mar 2022 | 241-0 v Celta VigoVillarreal 1-0 Celta Vigo |
| 20 | Sun 20 Mar 2022 | 240-1 v CádizCádiz 1-0 Villarreal |
| 21 | Sat 2 Apr 2022 | 240-2 v LevanteLevante 2-0 Villarreal |
| 22 | Sat 9 Apr 2022 | 24 1-1 v Athletic BilbaoVillarreal 1-1 Athletic Bilbao |
| 23 | Sat 16 Apr 2022 | 242-1 v GetafeGetafe 1-2 Villarreal |
| 24 | Sat 30 Apr 2022 | 241-2 v AlavésAlavés 2-1 Villarreal |
| 25 | Sun 8 May 2022 | 241-1 v SevillaVillarreal 1-1 Sevilla |
| 26 | Thu 12 May 2022 | 245-1 v Rayo VallecanoRayo Vallecano 1-5 Villarreal |
| 27 | Sun 15 May 2022 | 241-2 v Real SociedadVillarreal 1-2 Real Sociedad |
| 28 | Sun 22 May 2022 | 242-0 v BarcelonaBarcelona 0-2 Villarreal |
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