| 1 | Mon 16 Aug 2021 | 160-0 v GranadaVillarreal 0-0 Granada |
| 2 | Sat 21 Aug 2021 | 160-0 v EspanyolEspanyol 0-0 Villarreal |
| 3 | Sun 29 Aug 2021 | 162-2 v Atlético MadridAtlético Madrid 2-2 Villarreal |
| 4 | Sun 19 Sep 2021 | 16 0-0 v MallorcaMallorca 0-0 Villarreal |
| 5 | Wed 22 Sep 2021 | 164-1 v ElcheVillarreal 4-1 Elche |
| 6 | Sat 25 Sep 2021 | 160-0 v Real MadridReal Madrid 0-0 Villarreal |
| 7 | Tue 26 Oct 2021 | 163-3 v CádizVillarreal 3-3 Cádiz |
| 8 | Sat 30 Oct 2021 | 160-2 v ValenciaValencia 2-0 Villarreal |
| 9 | Sun 7 Nov 2021 | 161-0 v GetafeVillarreal 1-0 Getafe |
| 10 | Sat 20 Nov 2021 | 161-1 v Celta VigoCelta Vigo 1-1 Villarreal |
| 11 | Sat 4 Dec 2021 | 16 0-1 v SevillaSevilla 1-0 Villarreal |
| 12 | Sun 12 Dec 2021 | 162-0 v Rayo VallecanoVillarreal 2-0 Rayo Vallecano |
| 13 | Sat 18 Dec 2021 | 163-1 v Real SociedadReal Sociedad 1-3 Villarreal |
| 14 | Tue 21 Dec 2021 | 165-2 v AlavésVillarreal 5-2 Alavés |
| 15 | Mon 3 Jan 2022 | 165-0 v LevanteVillarreal 5-0 Levante |
| 16 | Sat 12 Feb 2022 | 160-0 v Real MadridVillarreal 0-0 Real Madrid |
| 17 | Sun 27 Feb 2022 | 165-1 v EspanyolVillarreal 5-1 Espanyol |
| 18 | Sat 5 Mar 2022 | 160-1 v OsasunaOsasuna 1-0 Villarreal |
| 19 | Sat 12 Mar 2022 | 161-0 v Celta VigoVillarreal 1-0 Celta Vigo |
| 20 | Sun 20 Mar 2022 | 160-1 v CádizCádiz 1-0 Villarreal |
| 21 | Tue 19 Apr 2022 | 162-0 v ValenciaVillarreal 2-0 Valencia |
| 22 | Sat 30 Apr 2022 | 16 1-2 v AlavésAlavés 2-1 Villarreal |
| 23 | Sun 8 May 2022 | 161-1 v SevillaVillarreal 1-1 Sevilla |
| 24 | Thu 12 May 2022 | 165-1 v Rayo VallecanoRayo Vallecano 1-5 Villarreal |
| 25 | Sun 15 May 2022 | 161-2 v Real SociedadVillarreal 1-2 Real Sociedad |
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