| 1 | Mon 16 Aug 2021 | 6 0-0 v GranadaVillarreal 0-0 Granada |
| 2 | Sat 21 Aug 2021 | 6 0-0 v EspanyolEspanyol 0-0 Villarreal |
| 3 | Sun 29 Aug 2021 | 62-2 v Atlético MadridAtlético Madrid 2-2 Villarreal |
| 4 | Sun 19 Sep 2021 | 60-0 v MallorcaMallorca 0-0 Villarreal |
| 5 | Wed 22 Sep 2021 | 64-1 v ElcheVillarreal 4-1 Elche |
| 6 | Sat 25 Sep 2021 | 60-0 v Real MadridReal Madrid 0-0 Villarreal |
| 7 | Sun 3 Oct 2021 | 6 2-0 v Real BetisVillarreal 2-0 Real Betis |
| 8 | Sun 17 Oct 2021 | 6 1-2 v OsasunaVillarreal 1-2 Osasuna |
| 9 | Sat 23 Oct 2021 | 61-2 v Athletic BilbaoAthletic Bilbao 2-1 Villarreal |
| 10 | Sat 30 Oct 2021 | 60-2 v ValenciaValencia 2-0 Villarreal |
| 11 | Sun 7 Nov 2021 | 61-0 v GetafeVillarreal 1-0 Getafe |
| 12 | Sat 27 Nov 2021 | 61-3 v BarcelonaVillarreal 1-3 Barcelona |
| 13 | Sat 4 Dec 2021 | 60-1 v SevillaSevilla 1-0 Villarreal |
| 14 | Sun 12 Dec 2021 | 62-0 v Rayo VallecanoVillarreal 2-0 Rayo Vallecano |
| 15 | Sat 18 Dec 2021 | 63-1 v Real SociedadReal Sociedad 1-3 Villarreal |
| 16 | Tue 21 Dec 2021 | 65-2 v AlavésVillarreal 5-2 Alavés |
| 17 | Sun 9 Jan 2022 | 62-2 v Atlético MadridVillarreal 2-2 Atlético Madrid |
| 18 | Sun 16 Jan 2022 | 6 0-1 v ElcheElche 1-0 Villarreal |
| 19 | Sun 6 Feb 2022 | 6 2-0 v Real BetisReal Betis 0-2 Villarreal |
| 20 | Sun 27 Feb 2022 | 65-1 v EspanyolVillarreal 5-1 Espanyol |
| 21 | Sat 5 Mar 2022 | 60-1 v OsasunaOsasuna 1-0 Villarreal |
| 22 | Sun 20 Mar 2022 | 6 0-1 v CádizCádiz 1-0 Villarreal |
| 23 | Sat 2 Apr 2022 | 60-2 v LevanteLevante 2-0 Villarreal |
| 24 | Sat 16 Apr 2022 | 62-1 v GetafeGetafe 1-2 Villarreal |
| 25 | Tue 19 Apr 2022 | 62-0 v ValenciaVillarreal 2-0 Valencia |
| 26 | Sat 30 Apr 2022 | 6 1-2 v AlavésAlavés 2-1 Villarreal |
| 27 | Sun 8 May 2022 | 6 1-1 v SevillaVillarreal 1-1 Sevilla |
| 28 | Thu 12 May 2022 | 65-1 v Rayo VallecanoRayo Vallecano 1-5 Villarreal |
| 29 | Sun 15 May 2022 | 61-2 v Real SociedadVillarreal 1-2 Real Sociedad |
| 30 | Sun 22 May 2022 | 62-0 v BarcelonaBarcelona 0-2 Villarreal |
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