| 1 | Mon 16 Aug 2021 | 7 0-0 v GranadaVillarreal 0-0 Granada |
| 2 | Sat 21 Aug 2021 | 70-0 v EspanyolEspanyol 0-0 Villarreal |
| 3 | Sun 29 Aug 2021 | 7 2-2 v Atlético MadridAtlético Madrid 2-2 Villarreal |
| 4 | Sun 17 Oct 2021 | 71-2 v OsasunaVillarreal 1-2 Osasuna |
| 5 | Sat 23 Oct 2021 | 71-2 v Athletic BilbaoAthletic Bilbao 2-1 Villarreal |
| 6 | Sat 4 Dec 2021 | 70-1 v SevillaSevilla 1-0 Villarreal |
| 7 | Sun 12 Dec 2021 | 72-0 v Rayo VallecanoVillarreal 2-0 Rayo Vallecano |
| 8 | Sat 18 Dec 2021 | 73-1 v Real SociedadReal Sociedad 1-3 Villarreal |
| 9 | Tue 21 Dec 2021 | 75-2 v AlavésVillarreal 5-2 Alavés |
| 10 | Mon 3 Jan 2022 | 75-0 v LevanteVillarreal 5-0 Levante |
| 11 | Sun 9 Jan 2022 | 72-2 v Atlético MadridVillarreal 2-2 Atlético Madrid |
| 12 | Sun 16 Jan 2022 | 70-1 v ElcheElche 1-0 Villarreal |
| 13 | Sun 6 Feb 2022 | 72-0 v Real BetisReal Betis 0-2 Villarreal |
| 14 | Sun 20 Mar 2022 | 70-1 v CádizCádiz 1-0 Villarreal |
| 15 | Sat 2 Apr 2022 | 70-2 v LevanteLevante 2-0 Villarreal |
| 16 | Sat 9 Apr 2022 | 71-1 v Athletic BilbaoVillarreal 1-1 Athletic Bilbao |
| 17 | Sat 16 Apr 2022 | 72-1 v GetafeGetafe 1-2 Villarreal |
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